In n = 1 RPP, the BA cations interlaced with one another a result of the interaction with apical I atom (shaded as pink) of surface PbI6 octahedron, where by a larger in-plane octahedral tilt and a small out-of-airplane tilt exist. In the case of n = four RPP, the BA molecules adopt a “head-to-head” configuration so that their NH3 group

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